Browsing by Autor "Patrick Ginot"

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Atmospheric warming at a high‐elevation tropical site revealed by englacial temperatures at Illimani, Bolivia (6340 m above sea level, 16°S, 67°W)
(American Geophysical Union, 2010) Adrien Gilbert; Patrick Wagnon; Christian Vincent; Patrick Ginot; M. Funk
In June 1999, a deep (138.7 m) ice core was extracted from the summit glacier of Illimani, Bolivia (6340 m above sea level, 16°39′S, 67°47′W), and an englacial temperature profile was measured in the borehole. Using on‐site and regional meteorological data as well as ice core stratigraphy, past surface temperatures were reconstructed with a heat flow model. The englacial temperature measurements exhibit a profile that is far from a steady state, reflecting an increasing atmospheric temperature over several years and nonstationary climatic conditions. Englacial temperature interpretation, using air temperature data, borehole temperature inversion, and melting rate quantification based on ice core density, shows two warming phases from 1900 to 1960 (+0.5 ± 0.3 K starting approximately in 1920–1930) and from 1985 to 1999 (+0.6 ± 0.2 K), corresponding to a mean atmospheric temperature rise of 1.1 ± 0.2 K over the 20th century. According to various climate change scenarios, the future evolution of englacial temperatures was simulated to estimate when and under what conditions this high‐elevation site on the Illimani summit glacier could become temperate in the future. Results show that this glacier might remain cold for more than 90 years in the case of a +2 K rise over the 21st century but could become temperate in the first 20 m depth between 2050 and 2060 if warming reaches +5 K.
Biomass-burning and urban emission impacts in the Andes Cordillera region based on in-situ measurements from the Chacaltaya observatory, Bolivia (5240 m a.s.l.)
(2019) Chauvigné Aurélien; Diego Aliaga; Marcos Andrade; Patrick Ginot; Radovan Krejčí; Griša Močnik; Nadège Montoux; Isabel Moreno; Thomas Müller; Marco Pandolfi
Abstract. We present the variability of aerosol particle optical properties measured at the global Atmosphere Watch (GAW) station Chacaltaya (5240 m a.s.l.). The in-situ mountain site is ideally located to study regional impacts of the densely populated urban area of La Paz/El Alto, and the intensive activity in the Amazonian basin. Four year measurements allow to study aerosol particle properties for distinct atmospheric conditions as stable and turbulent layers, different airmass origins, as well as for wet and dry seasons, including biomass-burning influenced periods. The absorption, scattering and extinction coefficients (median annual values of 0.74, 12.14 and 12.96 Mm−1 respectively) show a clear seasonal variation with low values during the wet season (0.57, 7.94 and 8.68 Mm−1 respectively) and higher values during the dry season (0.80, 11.23 and 14.51 Mm−1 respectively). These parameters also show a pronounced diurnal variation (maximum during daytime, minimum during night-time, as a result of the dynamic and convective effects of leading to lower atmospheric layers reaching the site during daytime. Retrieved intensive optical properties are significantly different from one season to the other, showing the influence of different sources of aerosols according to the season. Both intensive and extensive optical properties of aerosols were found to be different among the different atmospheric layers. The particle light absorption, scattering and extinction coefficients are in average 1.94, 1.49 and 1.55 times higher, respectively, in the turbulent layer compared to the stable layer. We observe that the difference is highest during the wet season and lowest during the dry season. Using wavelength dependence of aerosol particle optical properties, we discriminated contributions from natural (mainly mineral dust) and anthropogenic (mainly biomass-burning and urban transport or industries) emissions according to seasons and tropospheric layers. The main sources influencing measurements at CHC are arising from the urban area of La Paz/El Alto, and regional biomass-burning from the Amazonian basin. Results show a 28 % to 80 % increase of the extinction coefficients during the biomass-burning season with respect to the dry season, which is observed in both tropospheric layers. From this analyse, long-term observations at CHC provides the first direct evidence of the impact of emissions in the Amazonian basin on atmospheric optical properties far away from their sources, all the way to the stable layer.
CCN production by new particle formation in the free troposphere
(Copernicus Publications, 2017) Clémence Rose; Karine Sellegri; Isabel Moreno; Fernando Velarde; Michel Ramonet; Kay Weinhold; Radovan Krejčí; Marcos Andrade; Alfred Wiedensohler; Patrick Ginot
Abstract. Global models predict that new particle formation (NPF) is, in some environments, responsible for a substantial fraction of the total atmospheric particle number concentration and subsequently contributes significantly to cloud condensation nuclei (CCN) concentrations. NPF events were frequently observed at the highest atmospheric observatory in the world, on Chacaltaya (5240 m a.s.l.), Bolivia. The present study focuses on the impact of NPF on CCN population. Neutral cluster and Air Ion Spectrometer and mobility particle size spectrometer measurements were simultaneously used to follow the growth of particles from cluster sizes down to ∼ 2 nm up to CCN threshold sizes set to 50, 80 and 100 nm. Using measurements performed between 1 January and 31 December 2012, we found that 61 % of the 94 analysed events showed a clear particle growth and significant enhancement of the CCN-relevant particle number concentration. We evaluated the contribution of NPF, relative to the transport and growth of pre-existing particles, to CCN size. The averaged production of 50 nm particles during those events was 5072, and 1481 cm−3 for 100 nm particles, with a larger contribution of NPF compared to transport, especially during the wet season. The data set was further segregated into boundary layer (BL) and free troposphere (FT) conditions at the site. The NPF frequency of occurrence was higher in the BL (48 %) compared to the FT (39 %). Particle condensational growth was more frequently observed for events initiated in the FT, but on average faster for those initiated in the BL, when the amount of condensable species was most probably larger. As a result, the potential to form new CCN was higher for events initiated in the BL (67 % against 53 % in the FT). In contrast, higher CCN number concentration increases were found when the NPF process initially occurred in the FT, under less polluted conditions. This work highlights the competition between particle growth and the removal of freshly nucleated particles by coagulation processes. The results support model predictions which suggest that NPF is an effective source of CCN in some environments, and thus may influence regional climate through cloud-related radiative processes.
Climate variability during the last 1000 years inferred from Andean ice cores: A review of methodology and recent results
(Elsevier BV, 2008) Françoise Vimeux; Patrick Ginot; Margit Schwikowski; Mathias Vuille; Georg F. Hoffmann; Lonnie G. Thompson; U. Schotterer
Comment on acp-2022-780
(2023) Valeria MardoÃ±ez; Marco Pandolfi; Lucille Joanna S. Borlaza; Jean‐Luc Jaffrezo; AndrÃ©s Alastuey; Jean‐Luc Besombes; Isabel Moreno; Noemí Pérez; GriÅ¡a MoÄ nik; Patrick Ginot
Abstract. La Paz and El Alto are two fast-growing high-altitude Bolivian cities forming the second largest metropolitan area in the country, located between 3200 and 4050 m a.s.l. Together they host a growing population of around 1.8 million people. The air quality in this conurbation is strongly influenced by urbanization. However, there are no comprehensive studies that have assessed the sources of air pollution and their impacts on health. Despite being neighboring cities, the drastic change in altitude and topography between La Paz and El Alto together with different socio-economic activities lead to different sources, dynamics and transport of particulate matter (PM). In this investigation, PM10 samples were collected at two urban background stations located in La Paz and El Alto between April 2016 and June 2017. The samples were later analyzed for a wide range of chemical species including numerous source tracers (OC, EC, water-soluble ions, sugar anhydrides, sugar alcohols, trace metals, and molecular organic species). The US-EPA Positive Matrix Factorization (PMF v.5.0) receptor model was then applied for source apportionment of PM10. This is the first source apportionment study in South America that incorporates a large set of organic markers (such as levoglucosan, polycyclic aromatic hydrocarbons – PAH, hopanes and alkanes) together with inorganic species. The multisite PMF resolved 11 main sources of PM. The largest annual contribution to PM10 came from two major sources: the ensemble of the four vehicular emissions sources (exhaust and non-exhaust), together responsible for 35 % and 25 % of the measured PM in La Paz and El Alto, respectively, and dust contributing 20 % and 32 % to the total. Secondary aerosols contributed 22 % (24 %) in La Paz (El Alto). Agriculture-related smoke from biomass burning originated in the Bolivian lowlands and neighboring countries contributed to 8 % (7 %) of the total PM10 mass annually. This contribution increased to 17 % (13 %) between August–October. Primary biogenic emissions were responsible for 13 % (7 %) of the measured PM10 mass. Finally, it was possible to identify a profile related to open waste burning occurring between the months of May and August. Despite the fact that this source contributed only to 2 % (5 %) of the total PM10 mass, it constitutes the second largest source of PAHs, compounds potentially hazardous to health. Our analysis resulted in the identification of two specific traffic-related sources. In addition, we also identified a lubricant source (not frequently identified) and a non-exhaust emissions source. This study shows that PM10 concentrations in La Paz and El Alto region are mostly impacted by a limited number of local sources. In conclusion, dust, traffic emissions, open waste burning and biomass burning are the main sources to target in order to improve air quality in both cities.
Dust record in an ice core from tropical Andes (Nevado Illimani – Bolivia), potential for climate variability analyses in the Amazon basin
(2020) Filipe Gaudie Ley Lindau; Jefferson Cárdia Simões; Rafael da Rocha Ribeiro; Patrick Ginot; Barbara Delmonte; Giovanni Baccolo; Stanislav Kutuzov; Valter Maggi; Edson Ramírez
Abstract. Understanding the mechanisms controlling glacial retreat in the tropical Andes can strengthen future predictions of ice cover in the region. As glaciers are a dominant freshwater source in these regions, accurate ice cover predictions are necessary for developing effective strategies to protect future water resources. In this study, we investigated a 97-year dust record from two Nevado Illimani ice cores to determine the dominant factors controlling particle concentration and size distribution. In addition, we measured the area of a Nevado Illimani glacier (glacier n°8) using aerial photographs from 1956 and 2009. We identified two dustier periods during the 20th century (1930s–1940s and 1980s–2016), which were linked to reduced moisture transport from the Amazon basin. This promoted an unprecedented increase in the percentage of coarse dust particles (CPPn, ∅ > 10 μm) during the 1990s, as drier local conditions favored the emission and deposition of coarse particles on the glacier. Moisture advection from the Amazon basin to Nevado Illimani was influenced by tropical North Atlantic sea surface temperatures (TNA), which was supported by the correlation between TNA and CPPn (r = 0.52). Furthermore, glacial retreat has been accelerating since the 1980s, and a notable relationship between CPPn and the freezing level height (FLH, r = 0.41) was observed. This suggests that higher FLHs promote glacial retreat, which exposes fresh glacial sediments and facilitates the transport of coarse dust particles to the Nevado Illimani summit. Therefore, both the area of glacier n°8 and the ice core record of coarse dust particles were found to respond to climate variability—particularly to the warmer conditions across the southern tropical Andes and drier conditions over the Amazon basin.
Environmental records from temperate glacier ice on Nevado Coropuna saddle, southern Peru
(Copernicus Publications, 2009) J. Herreros; Isabel Moreno; Jean‐Denis Taupin; Patrick Ginot; Nicolas Patris; M. de Angelis; Marie‐Pierre Ledru; Fanny Delachaux; U. Schotterer
Abstract. We investigated past climate variability and the zonal short and long-range transport of air masses in tropical South America using chemical, isotopic and palynological signals from a 42 m-long ice core recovered in 2003 from the saddle of the Nevado Coropuna, southern Peru (72°39´ W; 15°32´ S; 6080 m a.s.l.). We found that precipitation at this site depends mainly on the easterly circulation of air masses originated from the tropical Atlantic Ocean. Nevertheless, sporadic Pacific air masses arrivals, and strong cold waves coming from southern South America reach this altitude site. In spite of post-depositional effects, we were able to identify two strong ENSO (El Niño-Southern Oscillation) event signatures (1982–1983 and 1992) and the eruptive activity of the nearby Sabancaya volcano (1994).
Frequent nucleation events at the high altitude station of Chacaltaya (5240 m a.s.l.), Bolivia
(Elsevier BV, 2014) Clémence Rose; Karine Sellegri; Fernando Velarde; Isabel Moreno; Michel Ramonet; Kay Weinhold; Radovan Krejčí; Patrick Ginot; Marcos Andrade; A. Wiedensohler
Glaciers and Climate in the Andes between the Equator and 30° S: What is Recorded under Extreme Environmental Conditions?
(Springer Nature (Netherlands), 2003) U. Schotterer; Martín Grosjean; Willibald Stichler; Patrick Ginot; C. Kull; H. Bonnaveira; Bernard Francou; H. W. Gäggeler; Robert Gallaire; Georg F. Hoffmann
New Particle Formation and impact on CCN concentrationsin the boundary layer and free troposphere at the highaltitude station of Chacaltaya (5240 m a.s.l.), Bolivia
(2016) Clémence Rose; Karine Sellegri; Isabel Moreno; Fernando Velarde; Michel Ramonet; Kay Weinhold; Radovan Krejčí; Marcos Andrade; Alfred Wiedensohler; Patrick Ginot
Abstract. Global models predict that new particle formation (NPF) is, in some environments, responsible for a substantial fraction of the total atmospheric particle number concentration and subsequently contribute significantly to cloud condensation nuclei (CCN) concentrations. NPF events were frequently observed at the highest atmospheric observatory in the world, Chacaltaya (5240 m a.s.l.), Bolivia. The present study focuses on the impact of NPF on CCN population. Neutral cluster and Air Ion Spectrometer and mobility particle size spectrometer measurements were simultaneously used to follow the growth of particles from cluster sizes down to ~ 2 nm up to CCN threshold sizes set to 50, 80 and 100 nm. Using measurements performed between January 1 and December 31 2012, we found that 61% of the 94 analysed events showed a clear particle growth and significant enhancement of the CCN-relevant particle number concentration. We evaluated the contribution of NPF events relative to the transport of pre-existing particles to the site. The averaged production of 50 nm particles during those events was 5072 cm−3, and 1481 cm−3 for 100 nm particles, with a larger contribution of NPF compared to transport, especially during the wet season. The data set was further segregated into boundary layer (BL) and free troposphere (FT) conditions at the site. The NPF frequency of occurrence was higher in the BL (48 %) compared to the FT (39 %). Particle condensational growth was more frequently observed for events initiated in the FT, but on average faster for those initiated in the BL, when the amount of condensable species was most probably larger. As a result, the potential to form new CCN was higher for events initiated in the BL (67 % against 56 % in the FT). In contrast, higher CCN number concentration increases were found when the NPF process initially occurred in the FT, under less polluted conditions. This work highlights the competition between particle growth and the removal of freshly nucleated particles by coagulation processes. The results support model predictions which suggest that NPF is an effective source of CCN in some environments, and thus may influence regional climate through cloud related radiative processes.
Potential for climate variability reconstruction from Andean glaciochemical records
(Cambridge University Press, 2002) Patrick Ginot; Margit Schwikowski; U. Schotterer; Willibald Stichler; H. W. Gäggeler; Bernard Francou; Robert Gallaire; Bernard Pouyaud
Abstract In order to select glacier sites suitable for the reconstruction of short-term climate variability, chemical constituents of shallow cores from Chimborazo, Ecuador, Illimani, Bolivia, and Cerro Tapado, Chile, were analyzed to determine if they represent the climate and atmospheric conditions of the particular area. Pronounced variations were observed in the Chimborazo core, which were attributed to the seasonal occurrence of wet and dry periods. Using chemical tracers, the Pacific and the Amazon basin were identified as the two principal sources of atmospheric moisture. In the Illimani record, seasonality is obvious but is less regular than in the Chimborazo core. Chemical tracers point to the Amazon basin as a moisture source. Post-depositional sublimation masks a possible atmospheric signal in the glaciochemical records from Cerro Tapado. the arid conditions and a prevailing high condensation level also cause little variability in the stable-isotope content. Irregular, more negative δ 18 O values occur during the humid phases of El Niño events. Despite alterations due to sublimation, chemical tracers indicate the Pacific Ocean as a main moisture source for precipitation preserved on Glaciar CerroTapado.
Source apportionment study on particulate air pollution in two high-altitude Bolivian cities: La Paz and El Alto
(Copernicus Publications, 2023) Valeria Mardóñez; Marco Pandolfi; Lucille Joanna S. Borlaza; Jean‐Luc Jaffrezo; Andrés Alástuey; Jean‐Luc Besombes; Isabel Moreno; Noemí Pérez; Griša Močnik; Patrick Ginot
Abstract. La Paz and El Alto are two fast-growing, high-altitude Bolivian cities forming the second-largest metropolitan area in the country. Located between 3200 and 4050 m a.s.l. (above sea level), these cities are home to a burgeoning population of approximately 1.8 million residents. The air quality in this conurbation is heavily influenced by urbanization; however, there are no comprehensive studies evaluating the sources of air pollution and their health impacts. Despite their proximity, the substantial variation in altitude, topography, and socioeconomic activities between La Paz and El Alto result in distinct sources, dynamics, and transport of particulate matter (PM). In this investigation, PM10 samples were collected at two urban background stations located in La Paz and El Alto between April 2016 and June 2017. The samples were later analyzed for a wide range of chemical species including numerous source tracers (OC, EC, water-soluble ions, sugar anhydrides, sugar alcohols, trace metals, and molecular organic species). The United States Environmental Protection Agency (U.S. EPA) Positive Matrix Factorization (PMF v.5.0) receptor model was employed for the source apportionment of PM10. This is one of the first source apportionment studies in South America that incorporates an extensive suite of organic markers, including levoglucosan, polycyclic aromatic hydrocarbons (PAHs), hopanes, and alkanes, alongside inorganic species. The multisite PMF resolved 11 main sources of PM. The largest annual contribution to PM10 came from the following two major sources: the ensemble of the four vehicular emissions sources (exhaust and non-exhaust), accountable for 35 % and 25 % of the measured PM in La Paz and El Alto, respectively; and dust, which contributed 20 % and 32 % to the total PM mass. Secondary aerosols accounted for 22 % (24 %) in La Paz (El Alto). Agricultural smoke resulting from biomass burning in the Bolivian lowlands and neighboring countries contributed to 9 % (8 %) of the total PM10 mass annually, increasing to 17 % (13 %) between August–October. Primary biogenic emissions were responsible for 13 % (7 %) of the measured PM10 mass. Additionally, a profile associated with open waste burning occurring from May to August was identified. Although this source contributed only to 2 % (5 %) of the total PM10 mass, it constitutes the second largest source of PAHs, which are compounds potentially hazardous to human health. Our analysis additionally resolved two different traffic-related factors, a lubricant source (not frequently identified), and a non-exhaust emissions source. Overall, this study demonstrates that PM10 concentrations in La Paz and El Alto region are predominantly influenced by a limited number of local sources. In conclusion, to improve air quality in both cities, efforts should primarily focus on addressing dust, traffic emissions, open waste burning, and biomass burning.
Source apportionment study on particulate air pollution in two high-altitude Bolivian cities: La Paz and El Alto
(2022) Valeria Mardóñez; Marco Pandolfi; Lucille Joanna S. Borlaza; Jean‐Luc Jaffrezo; Andrés Alástuey; Jean‐Luc Besombes; Isabel Moreno; Noemí Pérez; Griša Močnik; Patrick Ginot
Abstract. La Paz and El Alto are two fast-growing high-altitude Bolivian cities forming the second largest metropolitan area in the country, located between 3200 and 4050 m a.s.l. Together they host a growing population of around 1.8 million people. The air quality in this conurbation is strongly influenced by urbanization. However, there are no comprehensive studies that have assessed the sources of air pollution and their impacts on health. Despite being neighboring cities, the drastic change in altitude and topography between La Paz and El Alto together with different socio-economic activities lead to different sources, dynamics and transport of particulate matter (PM). In this investigation, PM10 samples were collected at two urban background stations located in La Paz and El Alto between April 2016 and June 2017. The samples were later analyzed for a wide range of chemical species including numerous source tracers (OC, EC, water-soluble ions, sugar anhydrides, sugar alcohols, trace metals, and molecular organic species). The US-EPA Positive Matrix Factorization (PMF v.5.0) receptor model was then applied for source apportionment of PM10. This is the first source apportionment study in South America that incorporates a large set of organic markers (such as levoglucosan, polycyclic aromatic hydrocarbons – PAH, hopanes and alkanes) together with inorganic species. The multisite PMF resolved 11 main sources of PM. The largest annual contribution to PM10 came from two major sources: the ensemble of the four vehicular emissions sources (exhaust and non-exhaust), together responsible for 35 % and 25 % of the measured PM in La Paz and El Alto, respectively, and dust contributing 20 % and 32 % to the total. Secondary aerosols contributed 22 % (24 %) in La Paz (El Alto). Agriculture-related smoke from biomass burning originated in the Bolivian lowlands and neighboring countries contributed to 8 % (7 %) of the total PM10 mass annually. This contribution increased to 17 % (13 %) between August–October. Primary biogenic emissions were responsible for 13 % (7 %) of the measured PM10 mass. Finally, it was possible to identify a profile related to open waste burning occurring between the months of May and August. Despite the fact that this source contributed only to 2 % (5 %) of the total PM10 mass, it constitutes the second largest source of PAHs, compounds potentially hazardous to health. Our analysis resulted in the identification of two specific traffic-related sources. In addition, we also identified a lubricant source (not frequently identified) and a non-exhaust emissions source. This study shows that PM10 concentrations in La Paz and El Alto region are mostly impacted by a limited number of local sources. In conclusion, dust, traffic emissions, open waste burning and biomass burning are the main sources to target in order to improve air quality in both cities.
Supplementary material to &quot;Dust record in an ice core from tropical Andes (Nevado Illimani – Bolivia), potential for climate variability analyses in the Amazon basin&quot;
(2020) Filipe Gaudie Ley Lindau; Jefferson Cárdia Simões; Rafael da Rocha Ribeiro; Patrick Ginot; Barbara Delmonte; Giovanni Baccolo; Stanislav Kutuzov; Valter Maggi; Edson Ramírez