Browsing by Autor "René Gutierrez"

Now showing 1 - 7 of 7

A decade of atmospheric composition observations in the undersampled Central Andes
(2022) Marcos Andrade; Diego Aliaga; Luis Blacutt; Ricardo Forno; René Gutierrez; Fernando Velarde; Isabel Moreno; Laura Ticona; Alfred Wiedensohler; Radovan Krejčí
&lt;p&gt;Ten years of almost continuous observations at the highest Global Atmosphere Watch Regional station in the world are presented here. The Chacaltaya observatory (5240 m asl, 16.3&amp;#186;S, 68.1&amp;#186;W) was set up in December 2011. It is currently the only operational station characterizing optical and chemical properties of climate-relevant aerosol and gases in Bolivia and in a radius of about 1500 kilometers from the station. The observations show a clear influence of the well-marked dry and wet meteorological seasons. In addition, the impact on the Andean mountains of long and mid-range transport of biomass burning products from the lowlands is clearly recorded in different parameters measured at the station. Furthermore, the nearby presence of the largest metropolitan area in the region (~1.8 million inhabitants) is observed almost on a daily basis, and therefore different campaigns were carried out to characterize the area and its influence on our measurements. Specific results from these campaigns are discussed elsewhere. Finally, the topographic complexity represents an important challenge for modeling efforts in order to understand sources and sinks (and associated processes) of the observed parameters, requiring not only high spatial resolution and the correct choice of model options, but a novel way of interpreting these results. The decade of collaboration of an international consortium made it possible to keep the station running successfully. The challenge is now to preserve its functioning for the coming decades in a region with historically few high-quality observations while disrupting environmental and socio-economic changes take place.&lt;/p&gt;
CAMPAÑA DE MEDICIONES ATMOSFÉRICAS EN LOS ANDES BOLIVIANOS REALIZADA POR EQUIPO ESTUDIANTIL BOLIVIANO-ESTADOUNIDENSE
(2024) David N. Whiteman; Marcos Andrade; Ricardo Forno; MAMANI-PACO; BLACUTT; René Gutierrez; Decker Guzmán Zabalaga
A student-focused field measurement campaign was held in the vicinity of Mt. Chacaltaya in the Bolivian Andes near the city of La Paz on May 24, 2022. The campaign was part of a program funded by the US Department of State, the main goal of which was to foster cultural and scientific exchange among Bolivian and US students. As part of this exchange, a group of eight Bolivian and four U.S. students worked together to plan and execute measurements which focused on quantifying the flow of particulate matter from the city of La Paz toward the summit of Mt. Chacaltaya, where the world’s highest elevation Global Atmosphere Watch site is located. Measurements were performed at three locations along a canyon that leads toward the summit of Mt. Chacaltaya and is a natural pathway for city-generated pollutants to travel toward the GAW station. The measurements indicated the presence of regular, solarheating-generated, downslope/upslope wind flow that aids the movement of particles near the mountain surface. The development of convection during the afternoon regularly decreased the concentrations measured at the surface and thus complicated the interpretation of particle flows. A novel, low-cost tethersonde apparatus was developed by members of the Laboratory for Atmospheric Physics (LFA) at the Universidad Mayor de San Andres (UM- ´ SA). Use of this tethersonde permitted vertical profiles of winds, temperature, pressure and relative humidity to be acquired thus allowing the investigation of the vertical structure of the transition between downslope and upslope flow. Outside of the measurement campaign, the students engaged in cultural activities together to enjoy local Bolivian sites and get to know each other better. One of the goals of the experiment was to increase interest in the atmospheric sciences among UMSA students. The results of a post-campaign survey indicate that participation in this joint field campaign has increased the number of physics students participating in the activities of the LFA at UMSA
Evidence for Interhemispheric Mercury Exchange in the Pacific Ocean Upper Troposphere
(Wiley, 2022) Alkuin Maximilian Koenig; Jeroen E. Sonke; Olivier Magand; Marcos Andrade; Isabel Moreno; Fernando Velarde; Ricardo Forno; René Gutierrez; Luis Blacutt; Paolo Laj
Abstract Even though anthropogenic mercury (Hg) emissions to the atmosphere are ∼2.5 times higher in the Northern Hemisphere (NH) than in the Southern Hemisphere (SH), atmospheric Hg concentrations in the NH are only ∼1.5 times higher than in the SH. Global Hg models attribute this apparent discrepancy to large SH oceanic Hg emissions or to interhemispheric exchange of Hg through the atmosphere. However, no observational data set exists to serve as a benchmark to validate whether these coarse‐resolution models adequately represent the complex dynamics of interhemispheric Hg exchange. During the 2015–2016 El Niño, we observed at mount Chacaltaya in the tropical Andes a ∼50% increase in ambient Hg compared to the year before, coinciding with a shift in synoptic transport pathways. Using this event as a case study, we investigate the impact of interhemispheric exchange on atmospheric Hg in tropical South America. We use HYSPLIT to link Hg observations to long‐range transport and find that the observed Hg increase relates strongly to air masses from the tropical Pacific upper troposphere (UT), a region directly impacted by interhemispheric exchange. Inclusion of the modeled seasonality of interhemispheric air mass exchange strengthens this relationship significantly. We estimate that interhemispheric exchange drives Hg seasonality in the SH tropical Pacific UT, with strongly enhanced Hg between July and October. We validate this seasonality with previously published aircraft Hg observations. Our results suggest that the transport of NH‐influenced air masses to tropical South America via the Pacific UT occurs regularly but became more detectable at Chacaltaya in 2015–2016 because of a westward shift in air mass origin.
Fractality in high energy cosmic rays
(Elsevier BV, 2003) N. Martinić; R. Ticona; I. Poma; F. Osco; René Gutierrez
Operadores diferenciales en Mathematica 2.22
(1998) René Gutierrez
Seasonal patterns of atmospheric mercury in tropical South America as inferred by a continuous total gaseous mercury record at Chacaltaya station (5240 m) in Bolivia
(Copernicus Publications, 2021) Alkuin Maximilian Koenig; Olivier Magand; Paolo Laj; Marcos Andrade; Isabel Moreno; Fernando Velarde; Grover Salvatierra; René Gutierrez; Luis Blacutt; Diego Aliaga
Abstract. High-quality atmospheric mercury (Hg) data are rare for South America, especially for its tropical region. As a consequence, mercury dynamics are still highly uncertain in this region. This is a significant deficiency, as South America appears to play a major role in the global budget of this toxic pollutant. To address this issue, we performed nearly 2 years (July 2014–February 2016) of continuous high-resolution total gaseous mercury (TGM) measurements at the Chacaltaya (CHC) mountain site in the Bolivian Andes, which is subject to a diverse mix of air masses coming predominantly from the Altiplano and the Amazon rainforest. For the first 11 months of measurements, we obtained a mean TGM concentration of 0.89±0.01 ng m−3, which is in good agreement with the sparse amount of data available from the continent. For the remaining 9 months, we obtained a significantly higher TGM concentration of 1.34±0.01 ng m−3, a difference which we tentatively attribute to the strong El Niño event of 2015–2016. Based on HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory) back trajectories and clustering techniques, we show that lower mean TGM concentrations were linked to either westerly Altiplanic air masses or those originating from the lowlands to the southeast of CHC. Elevated TGM concentrations were related to northerly air masses of Amazonian or southerly air masses of Altiplanic origin, with the former possibly linked to artisanal and small-scale gold mining (ASGM), whereas the latter might be explained by volcanic activity. We observed a marked seasonal pattern, with low TGM concentrations in the dry season (austral winter), rising concentrations during the biomass burning (BB) season, and the highest concentrations at the beginning of the wet season (austral summer). With the help of simultaneously sampled equivalent black carbon (eBC) and carbon monoxide (CO) data, we use the clearly BB-influenced signal during the BB season (August to October) to derive a mean TGM / CO emission ratio of (2.3±0.6)×10-7 ppbvTGM ppbvCO-1, which could be used to constrain South American BB emissions. Through the link with CO2 measured in situ and remotely sensed solar-induced fluorescence (SIF) as proxies for vegetation activity, we detect signs of a vegetation sink effect in Amazonian air masses and derive a “best guess” TGM / CO2 uptake ratio of 0.058 ±0.017 (ng m−3)TGM ppmCO2-1. Finally, significantly higher Hg concentrations in western Altiplanic air masses during the wet season compared with the dry season point towards the modulation of atmospheric Hg by the eastern Pacific Ocean.
Seasonal patterns of atmospheric mercury in tropical South America as inferred by a TGM continuous record at the Chacaltaya Station (5240 m) in Bolivia
(2020) Alkuin Maximilian Koenig; Olivier Magand; Paolo Laj; Marcos Andrade; Isabel Moreno; Fernando Velarde; Grover Salvatierra; René Gutierrez; Luis Blacutt; Diego Aliaga
Abstract. High-quality data of atmospheric mercury (Hg) is rare for South America, especially for its tropical part. In consequence, mercury dynamics are still highly uncertain in this region, a significant deficiency, as South America appears to play a major role in the global budget of this toxic pollutant. To address this issue, we performed nearly two years (July 2014–February 2016) of continuous high resolution total gaseous mercury (TGM) measurements at the Chacaltaya (CHC) mountain site in the Bolivian Andes, which is subject to a diverse mix of air masses coming predominantly from the Altiplano and the Amazon rainforest. For the first eleven months of measurements, we obtained a mean TGM concentration of 0.89±0.01 ng m−3, in good agreement with the sparse amount of data available from the continent. For the remaining nine months, we obtained a significantly higher TGM concentration of 1.34±0.01 ng m−3, a difference which we tentatively attribute to the strong El Niño event of 2015–2016. Based on HYSPLIT back-trajectories and clustering techniques, we show that lower mean TGM concentrations were linked to either westerly Altiplanic air masses or those originating from the lowlands to the south-east of CHC. Elevated TGM concentrations were related to northerly air masses of Amazonian or southerly air masses of Altiplanic origin, the former possibly linked to artisanal and small scale gold mining (ASGM), while the latter might be explained by volcanic activity. We observed a marked seasonal pattern, with low TGM concentrations in the dry season (austral winter), rising concentrations during biomass burning (BB) season, and highest concentrations at the beginning of the wet season (austral summer). With the help of simultaneously sampled equivalent black carbon (eBC) and carbon monoxide (CO) data, we use the clearly BB influenced signal during BB season (August to October) to derive a mean TGM/CO emission ratio of (2.3±0.6)·10−7 ppbvTGM ppbvCO−1, which could be used to constrain South American BB emissions. Through the link with in-situ measured CO2 and remotely sensed solar-induced fluorescence (SIF) as proxies for vegetation activity, we detect signs of a vegetation sink effect in Amazonian air masses and derive a best guess TGM/CO2 uptake ratio of 0.058±0.017 (ng m−3)TGM ppmCO2−1. Finally, significantly higher Hg concentrations in western Altiplanic air masses during the wet season as compared to the dry season point towards the modulation of atmospheric Hg by the Eastern Pacific Ocean.