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Browsing by Autor "Timothy J. Broderick"

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    <i>δ</i> <sup>13</sup> C methane source signatures from tropical wetland and rice field emissions
    (Royal Society, 2021) James L. France; Rebecca Fisher; David Lowry; Grant Allen; Marcos Andrade; Stéphane Bauguitte; Keith Bower; Timothy J. Broderick; M. C. Daly; Grant L. Forster
    The atmospheric methane (CH<sub>4</sub>) burden is rising sharply, but the causes are still not well understood. One factor of uncertainty is the importance of tropical CH<sub>4</sub> emissions into the global mix. Isotopic signatures of major sources remain poorly constrained, despite their usefulness in constraining the global methane budget. Here, a collection of new <i>δ</i><sup>13</sup>C<sub>CH<sub>4</sub></sub> signatures is presented for a range of tropical wetlands and rice fields determined from air samples collected during campaigns from 2016 to 2020. Long-term monitoring of <i>δ</i><sup>13</sup>C<sub>CH<sub>4</sub></sub> in ambient air has been conducted at the Chacaltaya observatory, Bolivia and Southern Botswana. Both long-term records are dominated by biogenic CH<sub>4</sub> sources, with isotopic signatures expected from wetland sources. From the longer-term Bolivian record, a seasonal isotopic shift is observed corresponding to wetland extent suggesting that there is input of relatively isotopically light CH<sub>4</sub> to the atmosphere during periods of reduced wetland extent. This new data expands the geographical extent and range of measurements of tropical wetland and rice <i>δ</i><sup>13</sup>C<sub>CH<sub>4</sub></sub> sources and hints at significant seasonal variation in tropical wetland <i>δ</i><sup>13</sup>C<sub>CH<sub>4</sub></sub> signatures which may be important to capture in future global and regional models. This article is part of a discussion meeting issue 'Rising methane: is warming feeding warming? (part 2)'.

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